Acquiring P.A. Semi got them Dan Dobberpuhl and Jim Keller, which laid a good design foundation. However, IMO, I'd lean towards these as the decisive factors today:
1) Apple's financial firepower allowing them to book out SOTA process nodes
2) Apple being less cost-sensitive in their designs vs. Qualcomm or Intel. Since Apple sells devices, they can justify 'expensive' decisions like massive caches that require significantly more die area.
P.A. Semi contributed greatly to Apple silicon, but the company has nothing to do with PA-RISC. In fact, their most notable chip before Apple bought them was Power ISA.